Polymer Nanocomposites and Properties Open access Peer reviewed

Reinforcing Effect of Two‐Dimensional Nano‐ OMMT Modifier in Polyvinyl Butyral

Haiyun Chen, Weimin Ye, Kunlun Wang, Yingliang Liu and 2 more

Journal of Applied Polymer Science | Oct 12, 2026

Abstract

Abstract

ABSTRACT To address the poor mechanical properties of polyvinyl butyral (PVB) and to deepen the understanding of the reinforcement mechanisms of nano materials in polymer matrices, this study reinforced PVB with a two‐dimensional (2D) nano‐organofunctionalized Montmorillonite (OMMT). To achieve proper performance of MMT in PVB, the MMT was functionalized using cocamidopropyl Betaine (CPB) and γ ‐(2, 3‐epoxypropoxy) propyl trimethoxy silane (KH560). By the method of in situ synthesis, the PVB/OMMT nanocomposites were prepared. The glass transition temperature ( T g ) of the PVB/OMMT‐0.30 resin was ~71°C, higher than that of neat PVB (~65°C). The PVB/OMMT‐0.20 nanocomposite film exhibited the highest tensile strength, right‐angle tear strength and max 180° peel strength against glass, together with a lower strain to failure, and it survived a falling‐ball impact without penetration. Rheological analysis confirmed that the storage and loss moduli of the matrix were improved, with PVB/OMMT‐0.20 showing the highest values. This work elucidates the effect of 2D nano‐OMMT on the performance of PVB resins and films and provides theoretical insight and technical guidance for the design and optimization of high‐performance PVB‐based composites.

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Authors

Researchers on this paper

Haiyun Chen

first | Zhengzhou University | ORCID 0009-0003-6063-5120

Weimin Ye

middle | Institute of New Materials

Kunlun Wang

middle | Zhengzhou University | ORCID 0000-0002-5371-8441

Yingliang Liu

middle | Zhengzhou University | ORCID 0000-0001-6515-165X

Qianyu Zhao

middle | Zhengzhou University | ORCID 0009-0003-0405-1884

Shaokui Cao

last | Zhengzhou University

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Citation

BibTeX

@article{Chen2026Reinforcing,
  title = {Reinforcing Effect of Two‐Dimensional Nano‐ OMMT Modifier in Polyvinyl Butyral},
  author = {Haiyun Chen and Weimin Ye and Kunlun Wang and Yingliang Liu and Qianyu Zhao and Shaokui Cao},
  journal = {Journal of Applied Polymer Science},
  year = {2026},
  doi = {10.1002/app.71611},
  url = {https://doi.org/10.1002/app.71611}
}

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